Since this is a larger landmass in Maine I got to thinking that the introduction to another vault is a strong possibility. Here is my experiment.
Residents inside are only able to communicate to each other using terminals. They never see each other at all. The catch is only once a year they can get together (to reproduce etc..) but then back to the rooms they are locked in. That is what they were told anyway, and soon will be a known lie. Plot twist is, the computer AI generates the fake one day event and the residents never leave the rooms. So they think they missed out. So you can tell they absolutely went crazy and all they had was the screens to entertain themselves, for better or worse.
Just an idea and like to hear what Vault-Tec experiment you want in Far Harbor!