Here is a list of minor things that could happen to make people upset, and a combination of them would make the people furious. First, bad forms of government (I'm not sure what NCR do): Monarchery, dictatorship, communism (maybe the NCR isn't communist, but the faction that wants to take over is. Communism does usually come around when an armed minority with help from outside resources, overthrows a majority. This is far from unheard of). Anything that gives them too much control and puts down too many restrictions. Strict rules that could be in effect: marriage laws, buying homes, curfew. Maybe they're doing something else the people don't like: lowering wages, raising taxes, raising overall prices, taking control of businesses (Like in New Vegas where it was hard to form your own business in Vegas), working in the black market, being too secretive (we can see people really don't like this, take Nixon for example), maybe even experimenting in nuclear explosives, round the clock guards on every semi-frequently traveled roads with heavy restrictions on gaining entrance, they could keep slaves from other factions to do their work (afterall they are the only major ones there), maybe evening buying/selling slaves that haven't done anything. All of these could be brought forth through paranoia, which isn't uncommon. With paranoia also comes: setting up spies all over the place to keep watch over you, strict rules regarding being though of as a traitor, bimonthly home checks for suspicious items. If someone is thought to be a traitor, they're punishment could be: Hanging, crucifiction, public punishment (like whipping), enslaving, toturing, beheading. Heck, they could even do these things to people who are actually innocent, only rumored to be a traitor, and you can hear their stories. With having heavy control of an area, you also get cocky. This can result in becoming over confident, thus military effectiveness can be decreased (though not by much). With confidance also comes the feeling that you're better than everyone else, which would make them treat the citizens like bums, low-lives, whimps, savages, etc, and actually call them names to their faces. They would have also had to form great enemies (even if we haven't heard of them) which would definetly help in a revolt. Any combination of these things would make the people furious, let's take H&H Tools (FO:NV) for example. If you read the terminals there, you find how heavy and unnecessary their restrictions were, and also how much the workers hated it. With enough of this, people will hate the NCR and will rise up against it. Over the 40 years we've heard few details on what's been going on in San Francisco, except NCR has major control, so we don't know what laws or regulations they could have put in place to tick people off. Though I agree the next game should take place somewhere else because people are tired of the NCR, I think San Fran. is a must for one of their future games. Hey, maybe by the time they're thinking of making it I'll be outta school and get hired by them, then I could assure you it would not be lame or stupid.
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Oh, yeah, time for school.