I'm jumping on the Muatra band-wagon. All of the Sermons get me going, but I especially enjoy the kinky bits
More seriously, stories of Shezarrines are great, and of course the whole cosmic drama with Lorkhan is appealing.
But what I like most are the mundane things. Little bits of history and culture and world-building that make TES unique to me.
I love the Khajiit's link to the moons and their institutionalized religious drug use. Khajiit and Ashlander culture, the aesthetics of Velothi design, a random stuff like "Who was Hestra and what were her accomplishments?" I find that piecing together a coherent world history out of miscellaneous mentions in various books is really fun!